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Composé binaire AB : ordre et désordre

dessin

Ordre ferromagnétique et désordre paramagnétique

dessin

Désordre réticulaire du type glace

dessin

Désordre topologique

dessin

Distribution radiale

graphique

Ordres à courte et à longue distance : variations

graphique

Tous les médias

Paramètres d'ordre à longue et courte distance

Revenons maintenant au type de désordre que nous avons qualifié de et cherchons à définir des paramètres susceptibles de le décrire quantitativement. Pour faire image, référons-nous au cas de l'alliage AB déjà évoqué et décrit dans la figure. Deux options peuvent être prises. La première consiste à s'intéresser au voisinage immédiat de chacun des atomes, c'est-à-dire à l', ou , comme nous venons de le faire dans le cas du désordre topologique. Soit Z le nombre de premiers voisins d'un site de la matrice. Supposons que ce site soit occupé par un atomeA, le nombre Z peut être divisé en deux parts: Z′ sites occupés par des atomesB et Z″ par des atomesA. Le rapport η=(Z′−Z″)/Z peut être utilisé pour décrire l'ordre local, les nombres Z′ et Z″ représentant les prises sur l'ensemble des sites de la matrice. η est appelé paramètre d'ordre à courte distance. Dans l'état parfaitement ordonné, on a Z′=Z et Z″=0, donc η=1. Dans l'état parfaitement désordonné, Z′=Z″, chaque site étant occupé avec la même probabilité par A ou B quel que soit son entourage, donc η=0. Dans tous les états intermédiaires, on a donc 0<η<1.

Mais le fait que, pour ce type de désordre, une matrice subsiste permet aussi de définir un . Désignons par α et β les réseaux formés respectivement par les sites occupés, d'une part, par les atomesA et, d'autre part, par les atomesB dans l'état ordonné. Dans un état désordonné, soit N le nombre d'atomesA occupant des sitesα (ou le nombre d'atomesB occupant des sitesβ), N le nombre d'atomesB occupant des sites α (ou le nombre d'atomesA occupant des sitesβ) et N=N+N le nombre total de sites. On définit le paramètre ξ d'ordre à grande distance par le rapport: ξ=(N−N)/N. Lorsque l'ordre est parfait (N=N, N=0), ξ=1; lorsque le désordre est statistiquement parfait dans l'ensemble de la matrice (N=N), ξ=0. Pour tous les états intermédiaires, 0<|ξ|<1.

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